Reversible Spin Textures with Giant Spin Splitting in Two-Dimensional Ga X Y (X= Se, Te; Y= Cl, Br, I) Compounds for A Persistent Spin Helix

Siti Amalia Sasmito, Muhammad Anshory, Ibnu Jihad, Moh. Adhib Ulil Absor

 

DOI: 10.1103/PhysRevB.104.115145

 

Journal : Physical Review B 104

Volume 104, September 2021, 115145

 

Abstract

The coexistence of ferroelectricity and spin-orbit coupling in noncentrosymmetric systems may allow for a nonvolatile control of spin textures in the momentum space by tuning the ferroelectric polarization. Based on first-principles calculations, supplemented with kp analysis, we report the emergence of the reversible spin textures in the two-dimensional (2D) GaXY (Se, Te; Cl, Br, I) monolayer compounds, a new class of 2D materials exhibiting in-plane ferroelectricity. We find that due to the large in-plane ferroelectric polarization, unidirectional out-of-plane spin textures are induced in the topmost valence band having giant spin splitting. Importantly, such out-of-plane spin textures, which can host a long-lived helical spin mode known as a persistent spin helix, can be fully reversed by switching the direction of the in-plane ferroelectric polarization. We show that the application of an external in-plane electric field oriented oppositely to the in-plane ferroelectric polarization direction is an effective method to flip the orientation of the out-of-plane spin textures. Thus, our findings can open avenues for interplay between the unidirectional out-of-plane spin textures and the in-plane ferroelectricity in 2D materials, which is useful for efficient and nonvolatile spintronic devices.

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